The role also gave the star her third Golden Globe and her second Screen Actors Guild statues.
Her first blockbuster, “Gone in 60 Seconds” was followed by 2001’s “Lara Croft: Tomb Raider,” giving Jolie her first major international hit.
Here's a recap of everything Us Weekly knows so far about Brangelina's shocking split.
The 52-year-old investigative journalist promises to expose the intimate details of the A-list Hollywood couple's marriage breakdown.
The relationship and marriage will be pulled apart in the documentary film by the bestselling author, and as the former couple embark on a high-profile divorce battle, the inside source cites that the film is the "last thing" they need.
The source said: "He and his team have also managed to acquire some never-before-seen footage and interviews with both Brad and Angelina.
A source told The Sun: "This is the definitive film about Brangelina and a lot of secrets are going to come out.
Ian has covered every cough and spit of their relationship and will reveal the real reasons behind Angelina filing for divorce."The biggest shock will be his claim that the couple were apart for more than a year prior to their break-up," they added.